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Impacts of Biomass Burning in Peninsular Southeast Asia on PM2.5 Concentration and Ozone Formation in Southern China During Springtime-A Case Study
Xing, Li1,2; Bei, Naifang3; Guo, Jianping4; Wang, Qiyuan2,5; Liu, Suixin2,5; Han, Yongming2,5; Pongpiachan, Siwatt6; Li, Guohui2,5
通讯作者Li, Guohui(ligh@ieecas.cn)
2021-11-27
发表期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
卷号126期号:22页码:16
摘要Biomass burning (BB) affects fine particulate matter (PM2.5) concentration and ozone (O-3) formation by emitting gaseous precursors and primary aerosols. The Impacts of BB in peninsular Southeast Asia (BB-PSEA) on PM2.5 concentration and O-3 formation in southern China are evaluated using a source-oriented WRF-Chem model to simulate an air pollution episode from March 21 to March 25, 2015. The source-oriented model separates the emissions from BB-PSEA and other sources and can evaluate the effects of aerosol-radiation interactions (ARIs) and aerosol-photolysis interactions (APIs) from BB-PSEA. Comparisons with observations reveal that the model performs well in simulating the air pollution episode. Sensitivity experiments show that BB-PSEA increases PM2.5 concentrations on the regional average by 39.3 mu g m(-3) (68.0%) in Yunnan Province (YNP) and 8.4 mu g m(-3) (24.1%) in other downwind areas (ODAs) in southern China, including the provinces of Guizhou, Guangxi, Hunan, Guangdong, Jiangxi, Fujian, and Zhejiang. PM2.5 enhancement is mainly attributed to primary aerosols in YNP and to secondary aerosols in ODA. BB-PSEA increases O-3 concentrations by 18.1 mu g m(-3) (19.4%) in YNP and decreases O-3 concentrations by 3.7 mu g m(-3) (5.3%) in ODA. The O-3 increase in YNP is attributed to the gaseous emissions of BB-PSEA, and the O-3 decrease in ODA is caused by the effects of ARI and API from BB-PSEA. NH3 emissions from BB-PSEA play a key role in enhancing secondary inorganic aerosols in southern China and determining increases in PM2.5 concentrations in ODA.
关键词biomass burning southeast Asia WRF-Chem aerosol-radiation feedback aerosol-photolysis interactions
DOI10.1029/2021JD034908
关键词[WOS]ORGANIC AEROSOL FORMATION ; TIANJIN-HEBEI BTH ; MEXICO-CITY ; SOURCE APPORTIONMENT ; PARTICULATE MATTER ; SOUTHWEST CHINA ; WINTERTIME HAZE ; SURFACE OZONE ; HONO SOURCES ; CHEM MODEL
收录类别SCI ; SCI
语种英语
资助项目Strategic Priority Research Program of the Chinese Academy of Sciences[XDB40030203] ; National Natural Science Foundation of China[41807310] ; National Natural Science Foundation of China[41661144020] ; Fundamental Research Funds for the Central Universities[GK202003066] ; Natural Science Foundation of Shaanxi Province[2020JQ-414]
WOS研究方向Meteorology & Atmospheric Sciences
项目资助者Strategic Priority Research Program of the Chinese Academy of Sciences ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Natural Science Foundation of Shaanxi Province
WOS类目Meteorology & Atmospheric Sciences
WOS记录号WOS:000723100300009
出版者AMER GEOPHYSICAL UNION
引用统计
被引频次:13[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/17276
专题粉尘与环境研究室
第四纪科学与全球变化卓越创新中心
通讯作者Li, Guohui
作者单位1.Shaanxi Normal Univ, Sch Geog & Tourism, Xian, Peoples R China
2.Chinese Acad Sci, Inst Earth Environm, SKLLQG, Xian, Peoples R China
3.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian, Peoples R China
4.Chinese Acad Meteorol Sci, State Key Lab Severe Weather, Beijing, Peoples R China
5.CAS Ctr Excellence Quaternary Sci & Global Change, Xian, Peoples R China
6.Natl Inst Dev Adm, Sch Social & Environm Dev, Bangkok, Thailand
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Xing, Li,Bei, Naifang,Guo, Jianping,et al. Impacts of Biomass Burning in Peninsular Southeast Asia on PM2.5 Concentration and Ozone Formation in Southern China During Springtime-A Case Study[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2021,126(22):16.
APA Xing, Li.,Bei, Naifang.,Guo, Jianping.,Wang, Qiyuan.,Liu, Suixin.,...&Li, Guohui.(2021).Impacts of Biomass Burning in Peninsular Southeast Asia on PM2.5 Concentration and Ozone Formation in Southern China During Springtime-A Case Study.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,126(22),16.
MLA Xing, Li,et al."Impacts of Biomass Burning in Peninsular Southeast Asia on PM2.5 Concentration and Ozone Formation in Southern China During Springtime-A Case Study".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 126.22(2021):16.
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