Impacts of Biomass Burning in Peninsular Southeast Asia on PM2.5 Concentration and Ozone Formation in Southern China During Springtime-A Case Study | |
Xing, Li1,2; Bei, Naifang3; Guo, Jianping4; Wang, Qiyuan2,5; Liu, Suixin2,5; Han, Yongming2,5; Pongpiachan, Siwatt6; Li, Guohui2,5 | |
通讯作者 | Li, Guohui(ligh@ieecas.cn) |
2021-11-27 | |
发表期刊 | JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES |
ISSN | 2169-897X |
卷号 | 126期号:22页码:16 |
摘要 | Biomass burning (BB) affects fine particulate matter (PM2.5) concentration and ozone (O-3) formation by emitting gaseous precursors and primary aerosols. The Impacts of BB in peninsular Southeast Asia (BB-PSEA) on PM2.5 concentration and O-3 formation in southern China are evaluated using a source-oriented WRF-Chem model to simulate an air pollution episode from March 21 to March 25, 2015. The source-oriented model separates the emissions from BB-PSEA and other sources and can evaluate the effects of aerosol-radiation interactions (ARIs) and aerosol-photolysis interactions (APIs) from BB-PSEA. Comparisons with observations reveal that the model performs well in simulating the air pollution episode. Sensitivity experiments show that BB-PSEA increases PM2.5 concentrations on the regional average by 39.3 mu g m(-3) (68.0%) in Yunnan Province (YNP) and 8.4 mu g m(-3) (24.1%) in other downwind areas (ODAs) in southern China, including the provinces of Guizhou, Guangxi, Hunan, Guangdong, Jiangxi, Fujian, and Zhejiang. PM2.5 enhancement is mainly attributed to primary aerosols in YNP and to secondary aerosols in ODA. BB-PSEA increases O-3 concentrations by 18.1 mu g m(-3) (19.4%) in YNP and decreases O-3 concentrations by 3.7 mu g m(-3) (5.3%) in ODA. The O-3 increase in YNP is attributed to the gaseous emissions of BB-PSEA, and the O-3 decrease in ODA is caused by the effects of ARI and API from BB-PSEA. NH3 emissions from BB-PSEA play a key role in enhancing secondary inorganic aerosols in southern China and determining increases in PM2.5 concentrations in ODA. |
关键词 | biomass burning southeast Asia WRF-Chem aerosol-radiation feedback aerosol-photolysis interactions |
DOI | 10.1029/2021JD034908 |
关键词[WOS] | ORGANIC AEROSOL FORMATION ; TIANJIN-HEBEI BTH ; MEXICO-CITY ; SOURCE APPORTIONMENT ; PARTICULATE MATTER ; SOUTHWEST CHINA ; WINTERTIME HAZE ; SURFACE OZONE ; HONO SOURCES ; CHEM MODEL |
收录类别 | SCI ; SCI |
语种 | 英语 |
资助项目 | Strategic Priority Research Program of the Chinese Academy of Sciences[XDB40030203] ; National Natural Science Foundation of China[41807310] ; National Natural Science Foundation of China[41661144020] ; Fundamental Research Funds for the Central Universities[GK202003066] ; Natural Science Foundation of Shaanxi Province[2020JQ-414] |
WOS研究方向 | Meteorology & Atmospheric Sciences |
项目资助者 | Strategic Priority Research Program of the Chinese Academy of Sciences ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Natural Science Foundation of Shaanxi Province |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS记录号 | WOS:000723100300009 |
出版者 | AMER GEOPHYSICAL UNION |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.ieecas.cn/handle/361006/17276 |
专题 | 粉尘与环境研究室 第四纪科学与全球变化卓越创新中心 |
通讯作者 | Li, Guohui |
作者单位 | 1.Shaanxi Normal Univ, Sch Geog & Tourism, Xian, Peoples R China 2.Chinese Acad Sci, Inst Earth Environm, SKLLQG, Xian, Peoples R China 3.Xi An Jiao Tong Univ, Sch Human Settlements & Civil Engn, Xian, Peoples R China 4.Chinese Acad Meteorol Sci, State Key Lab Severe Weather, Beijing, Peoples R China 5.CAS Ctr Excellence Quaternary Sci & Global Change, Xian, Peoples R China 6.Natl Inst Dev Adm, Sch Social & Environm Dev, Bangkok, Thailand |
推荐引用方式 GB/T 7714 | Xing, Li,Bei, Naifang,Guo, Jianping,et al. Impacts of Biomass Burning in Peninsular Southeast Asia on PM2.5 Concentration and Ozone Formation in Southern China During Springtime-A Case Study[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2021,126(22):16. |
APA | Xing, Li.,Bei, Naifang.,Guo, Jianping.,Wang, Qiyuan.,Liu, Suixin.,...&Li, Guohui.(2021).Impacts of Biomass Burning in Peninsular Southeast Asia on PM2.5 Concentration and Ozone Formation in Southern China During Springtime-A Case Study.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,126(22),16. |
MLA | Xing, Li,et al."Impacts of Biomass Burning in Peninsular Southeast Asia on PM2.5 Concentration and Ozone Formation in Southern China During Springtime-A Case Study".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 126.22(2021):16. |
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