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Level, distribution and sources of plutonium in the northeast and north China
Zhang, Weichao1,2; Hou, Xiaolin1,3,4,5; Zhang, Haitao2; Wang, Yanyun1; Dang, Haijun2; Xing, Shan1; Chen, Ning1
通讯作者Hou, Xiaolin(xiho@env.dtu.dk)
2021-11-15
发表期刊ENVIRONMENTAL POLLUTION
ISSN0269-7491
卷号289页码:9
摘要Concentrations of 239Pu and 240Pu in 163 surface soil samples and five soil cores collected from the northeast and north China were analyzed using the radiochemical separation combined with inductively coupled plasma mass spectrometry measurement. The average 240Pu/239Pu atomic ratios (0.185 +/- 0.018) for all surface soil samples indicated that the global fallout is the major source of plutonium in the studied region. The 239,240Pu concentrations of the surface soil ranged from 0.002 mBq/g to 4.82 mBq/g, lying in the range of the reported results in the areas with similar latitude, except for a few samples. The distribution of 239,240Pu in this region is controlled by the deposition of plutonium in the atmosphere and its preservation in the soil, which were affects by multifactors such as topography, climate, utilization of the land and vegetation coverage. The analytical results could be used as the baseline data for the assessment of the impact of nuclear activities in the past and the future.
关键词Plutonium isotopes Sources Distribution Environmental radioactivity Northeast and north China
DOI10.1016/j.envpol.2021.117967
关键词[WOS]LOESS PLATEAU ; PU ISOTOPES ; VERTICAL DISTRIBUTIONS ; SOIL-EROSION ; SEDIMENTS ; CHERNOBYL ; PU-240 ; CS-137 ; RADIONUCLIDES ; PU-240/PU-239
收录类别SCI ; SCI
语种英语
资助项目Chinese Academy of Sciences[132B61KYSB20180003] ; Chinese Academy of Sciences[XDB40020400] ; China Postdoctoral Science Foundation[2020M683759] ; Ministry of Science and Technology of China[2015FY110800] ; National Natural Science Foundation of China[11875261] ; National Natural Science Foundation of China[91643206] ; State Key Laboratory of Loess and Quaternary Geology[SKLLQG1927]
WOS研究方向Environmental Sciences & Ecology
项目资助者Chinese Academy of Sciences ; China Postdoctoral Science Foundation ; Ministry of Science and Technology of China ; National Natural Science Foundation of China ; State Key Laboratory of Loess and Quaternary Geology
WOS类目Environmental Sciences
WOS记录号WOS:000697048700005
出版者ELSEVIER SCI LTD
引用统计
被引频次:12[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/17038
专题加速器质谱中心
第四纪科学与全球变化卓越创新中心
通讯作者Hou, Xiaolin
作者单位1.Chinese Acad Sci, Inst Earth Environm, Xian AMS Ctr,State Key Lab Loess & Quaternary Geo, Shaanxi Key Lab Accelerator Mass Spectrometry Tec, Xian 710061, Peoples R China
2.Northwest Inst Nucl Technol, Xian 710024, Peoples R China
3.Tech Univ Denmark, Dept Environm Engn, Riso Campus, DK-4000 Roskilde, Denmark
4.CAS Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Peoples R China
5.Pilot Natl Lab Marine Sci & Technol Qingdao, Open Studio Ocean Continental Climate & Environm, Qingdao 266061, Peoples R China
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GB/T 7714
Zhang, Weichao,Hou, Xiaolin,Zhang, Haitao,et al. Level, distribution and sources of plutonium in the northeast and north China[J]. ENVIRONMENTAL POLLUTION,2021,289:9.
APA Zhang, Weichao.,Hou, Xiaolin.,Zhang, Haitao.,Wang, Yanyun.,Dang, Haijun.,...&Chen, Ning.(2021).Level, distribution and sources of plutonium in the northeast and north China.ENVIRONMENTAL POLLUTION,289,9.
MLA Zhang, Weichao,et al."Level, distribution and sources of plutonium in the northeast and north China".ENVIRONMENTAL POLLUTION 289(2021):9.
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