Interactive assessment of lignite and bamboo-biochar for geochemical speciation, modulation and uptake of Cu and other heavy metals in the copper mine tailing
Munir, Mehr Ahmed Mujtaba1,2,3; Irshad, Samina2,3; Yousaf, Balal2,3,4; Ali, Muhammad Ubaid5,6; Dan, Chen1; Abbas, Qumber7; Liu, Guijian2,3; Yang, Xiaoe1
通讯作者Liu, Guijian(lgj@ustc.edu.cn)
2021-07-20
发表期刊SCIENCE OF THE TOTAL ENVIRONMENT
ISSN0048-9697
卷号779页码:13
摘要This study was designed to examine the combined effect of bamboo-biochar (BC) and water-washed lignite (LGT) at copper mine tailings (CuMT) sites on the concentration of Cu and other metals in pore water (PW), their bioavailability, and change in geochemical speciation. Rapeseed (first cropping-season) and wheat (second cropping-season) were grown for 40-days each and the influence of applied-amendments on both cropping seasons was observed and compared. A significant increase in pH, water holding capacity (WHC), and soil organic carbon (SOC) was observed after the applied amendments in second cropping-seasons. The BC-LGT significantly reduced the concentration of Cu in PW after second cropping seasons; however, the concentration of Pb and Zn were increased with the individual application of biochar and LGT, respectively. BC-LGT and BC-2% significantly reduced the bioavailability of Cu and other HMs in both cropping seasons. The treated-CuMT was subjected to spectroscopic investigation through X-ray photoelectron spectroscopy (XPS), Fourier transform Infrared spectroscopy (FTIR), and X-ray powder diffraction (XRD). The results showed that Cu sorption mainly involved the coordination with hydroxyl and carboxyl functional groups, as well as the co-precipitation or complexation on mineral surfaces, which vary with the applied amendment and bulk amount of Mg, Mn, and Fe released during sorption-process. The co-application of BC-LGT exerted significant effectiveness in immobilizing Cu and other HMs in CuMT. The outcomes of the study indicated that co-application of BC-LGT is an efficacious combination of organic and inorganic materials for Cu adsorption which may provide some new information for the sustainable remediation of copper mine tailing. (c) 2021 Elsevier B.V. All rights reserved.
关键词Biochar Lignite Heavy metals Spectroscopic investigation
DOI10.1016/j.scitotenv.2021.146536
关键词[WOS]CONTAMINATED SOIL ; TRACE-ELEMENTS ; SEWAGE-SLUDGE ; RICE STRAW ; FLY-ASH ; MOBILITY ; LEAD ; IMMOBILIZATION ; AVAILABILITY ; COMPOST
收录类别SCI ; SCI
语种英语
资助项目National Natural Science Foundation of China[41173032] ; Key research and development projects of Anhui Province[1804b06020358]
WOS研究方向Environmental Sciences & Ecology
项目资助者National Natural Science Foundation of China ; Key research and development projects of Anhui Province
WOS类目Environmental Sciences
WOS记录号WOS:000655679800003
出版者ELSEVIER
引用统计
被引频次:24[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ieecas.cn/handle/361006/16697
专题黄土与第四纪地质国家重点实验室(2010~)
通讯作者Liu, Guijian
作者单位1.Zhejiang Univ, Coll Environm Resource Sci, Minist Educ, Key Lab Environm Remediat & Ecol Hlth, Zijingang Campus,Yuhangtang Rd 866, Hangzhou 310058, Peoples R China
2.Univ Sci & Technol China, Sch Earth & Space Sci, CAS Key Lab Crust Mantle Mat & Environm, Hefei 230026, Anhui, Peoples R China
3.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710075, Shaanxi, Peoples R China
4.Middle East Tech Univ, Environm Engn Dept, TR-06800 Ankara, Turkey
5.Southern Univ Sci & Technol, Sch Environm Sci & Engn, Guangdong Prov Key Lab Soil & Groundwater Pollut, Shenzhen 518000, Peoples R China
6.Southern Univ Sci & Technol, Sch Environm Sci & Engn, State Environm Protect Key Lab Integrated Surface, Shenzhen 518000, Peoples R China
7.Xi An Jiao Tong Univ, Dept Environm Sci & Engn, Xian 710049, Peoples R China
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Munir, Mehr Ahmed Mujtaba,Irshad, Samina,Yousaf, Balal,et al. Interactive assessment of lignite and bamboo-biochar for geochemical speciation, modulation and uptake of Cu and other heavy metals in the copper mine tailing[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2021,779:13.
APA Munir, Mehr Ahmed Mujtaba.,Irshad, Samina.,Yousaf, Balal.,Ali, Muhammad Ubaid.,Dan, Chen.,...&Yang, Xiaoe.(2021).Interactive assessment of lignite and bamboo-biochar for geochemical speciation, modulation and uptake of Cu and other heavy metals in the copper mine tailing.SCIENCE OF THE TOTAL ENVIRONMENT,779,13.
MLA Munir, Mehr Ahmed Mujtaba,et al."Interactive assessment of lignite and bamboo-biochar for geochemical speciation, modulation and uptake of Cu and other heavy metals in the copper mine tailing".SCIENCE OF THE TOTAL ENVIRONMENT 779(2021):13.
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